00:00 15-05-2007

In this talk, I will review Intracavity Laser Absorption
Spectroscopy  and  Cavity  Ringdown  Laser Absorption Spectroscopy
techniques applied to a study of combustion mechanisms. The use of
ultrasensitive Laser Absorption Methods allowed  us  to perform in
situ spatial  concentration  measurements  of HCO, 1CH2, OH and CH
radicals in  a low-pressure flat methane/air flame, and NH and NH2
in N2O doped low-pressure flat methane/air flame,  and compare the
results with model calculations.  Understanding  the mechanisms of
combustion  is  of  high  importance  to  the  mankind. Combustion
processes are largest universal source of energy. At the same time,
combustion  processes  are  largest  source  of  global  pollution.
Absolute concentration measurements  of  intermediate  species  of
combustion mechanism are necessary both  for determination of rate
constants of radical-radical reactions  and for better understand-
ing of the chemical mechanisms of combustion. One of the best ways
to improve the understanding of those mechanisms is  monitoring in
situ  of  spatial  concentration  profiles  of  different reactive
intermediates  followed  by  comparison  of the results with model

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